... anyone think you could use SharePoint Online with ArcGIS Online. Connecting the two via ArcGIS for SharePoint?
As far as I'm aware, there are no plans to integrate ArcGIS Online with SharePoint Online. ArcGIS for SharePoint is a client application that can work with SharePoint data + web services from ArcGIS Server and Web Maps from ArcGIS Online. In its current form it can't bridge the two different online platforms.
Hope this helps,
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This capability is expected later this month with the 4.1 release of Esri Maps for SharePoint. Keep your eyes posted for the announcement!
Esri HHS Account Manager
Yes, however I there were some bugs with 4.0, and since 4.1 is expected later this month, it's advisable to wait for it.